How Photoinduced Gate Screening and Leakage Currents Dynamically Change the Fermi Level in 2D Materials

physica status solidi (RRL) - Rapid Research Letters, vol. 14

Abstract

An in‐depth analysis of physics in 2D materials like transition metal dichalcogenides requires the measurement of many material properties as a function of Fermi level position within the electronic band structure. This is normally done by changing the charge carrier density of the 2D material via the gate electric field effect. Herein, a comparison of gate‐dependent measurements, which are acquired under different measurement conditions, is shown to encounter significant problems due to the temporal evolution of the charging of trap states inside the dielectric layer or at its interfaces. The impact of, e.g., the gate sweep direction and the sweep rate on the overall gate dependence gets especially prominent in optical measurements due to photoexcitation of donor and acceptor states. Under such conditions, the same nominal gate voltage may lead to different gate‐induced charge carrier densities and, hence, Fermi level positions. It is demonstrated that a current flow from or even through the dielectric layer via leakage currents can significantly diminish the gate tunability in optical measurements of 2D materials.

Authors 5

1. Frank Volmer Aachen 2nd Institute of Physics and JARA-FIT

   RWTH Aachen University · Jülich Aachen Research Alliance

   Affiliation as printed

   2nd Institute of Physics and JARA-FIT RWTH Aachen University 52074 Aachen Germany

2. Manfred Ersfeld Aachen 2nd Institute of Physics and JARA-FIT

   RWTH Aachen University · Jülich Aachen Research Alliance

   Affiliation as printed

   2nd Institute of Physics and JARA-FIT RWTH Aachen University 52074 Aachen Germany

3. Lars Rathmann Aachen 2nd Institute of Physics and JARA-FIT

   RWTH Aachen University · Jülich Aachen Research Alliance

   Affiliation as printed

   2nd Institute of Physics and JARA-FIT RWTH Aachen University 52074 Aachen Germany

4. Maximilian Heithoff Aachen 2nd Institute of Physics and JARA-FIT

   RWTH Aachen University · Jülich Aachen Research Alliance

   Affiliation as printed

   2nd Institute of Physics and JARA-FIT RWTH Aachen University 52074 Aachen Germany

5. Luca Kotewitz Aachen 2nd Institute of Physics and JARA-FIT

   RWTH Aachen University · Jülich Aachen Research Alliance

   Affiliation as printed

   2nd Institute of Physics and JARA-FIT RWTH Aachen University 52074 Aachen Germany