Comment on egusphere-2026-3954

Abstract

Abstract. How aerosol physicochemical properties affect aerosol-cloud interactions (ACI) and when these impacts are most pronounced represent an important source of ACI uncertainty. Targeting a representative liquid-phase cloud case over the Eastern China Ocean (ECO) under the winter monsoon featuring abundant meteorological, aerosol, and cloud variations, this study investigates the impacts of changes in aerosol size (volume-mean radius increased by 1.2 times and decreased by 45 %) and hygroscopicity (volume-mean hygroscopicity increased by 2.2 times and decreased by 62 %) using a spectral-bin cloud model. Results indicate that increased aerosol size and hygroscopicity generally enhance cloud development, raising the ECO-averaged cloud droplet number concentration (Nd) by 92 % and 53 %, respectively. These impacts peak under moderate aerosol concentrations (Na) and cold advection, where Nd increases up to 10-fold. Concurrently, increased aerosol size raises cloud water by 1.3 times and extends cloud lifetime by 85 %, whereas increased hygroscopicity has a much weaker effect. By contrast, decreased aerosol size and hygroscopicity generally suppress cloud development, reducing the ECO-averaged Nd by 49 % and 43 %, respectively. The former has a relatively strong impact, which is most notable in moderate-to-high Na environments under cold advection, reducing Nd and cloud water by over 80 % and 50 %, respectively. While changes in aerosol size generally exert a stronger overall impact than changes in hygroscopicity, specific conditions reveal the opposite. Notably, the enhancement of Nd by increased hygroscopicity under high Na, and the preservation of cloud and rainwater through evaporation suppression by decreased hygroscopicity, both surpass the effects caused by corresponding aerosol size changes.

Authors 6

1. Jianqi Zhao

   China Meteorological Administration · Nanjing University of Information Science and Technology

   Affiliation as printed

   China Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, China

2. Xiaoyan Ma corresponding

   China Meteorological Administration · Nanjing University of Information Science and Technology

   Affiliation as printed

   China Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, China

3. Hailing Jia Aachen SRON Netherlands Institute for Space Research

   Space Research Organisation Netherlands

   Affiliation as printed

   SRON Netherlands Institute for Space Research, Niels Bohrweg 4, 2333 CA Leiden, the Netherlands

4. Tong Yang

   China Meteorological Administration · Nanjing University of Information Science and Technology

   Affiliation as printed

   China Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, China

5. Peili Zou

   China Meteorological Administration · Nanjing University of Information Science and Technology

   Affiliation as printed

   China Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, China

6. Yingying Ku

   China Meteorological Administration · Nanjing University of Information Science and Technology

   Affiliation as printed

   China Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, China