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Short‐Term Tests, Long‐Term Predictions – Accelerating Ageing Characterisation of Lithium‐Ion Batteries

Batteries & Supercaps, vol. 7

Abstract

Abstract For the battery industry, quick determination of the ageing behaviour of lithium‐ion batteries is important both for the evaluation of existing designs as well as for R&D on future technologies. However, the target battery lifetime is 8–10 years, which implies low ageing rates that lead to an unacceptably long ageing test duration under real operation conditions. Therefore, ageing characterisation tests need to be accelerated to obtain ageing patterns in a period ranging from a few weeks to a few months. Known strategies, such as increasing the severity of stress factors, for example, temperature, current, and taking measurements with particularly high precision, need care in application to achieve meaningful results. We observe that this challenge does not receive enough attention in typical ageing studies. Therefore, this review introduces the definition and challenge of accelerated ageing along existing methods to accelerate the characterisation of battery ageing and lifetime modelling. We systematically discuss approaches along the existing literature. In this context, several test conditions and feasible acceleration strategies are highlighted, and the underlying modelling and statistical perspective is provided. This makes the review valuable for all who set up ageing tests, interpret ageing data, or rely on ageing data to predict battery lifetime.

Authors 20

  1. Karlsruhe Institute of Technology · Jülich Aachen Research Alliance · Imperial College London · RWTH Aachen University

    Affiliation as printed

    Chair for Electrochemical Energy Conversion and Storage Systems Institute for Power Electronics and Electrical Drives (ISEA) RWTH Aachen University CampusBoulevard 89 52074 Aachen Germany

    Institute of Thermal Process Engineering (TVT) Karlsruhe Institute of Technology (KIT) Germany

    Jülich Aachen Research Alliance JARA-Energy Templergraben 55 52056 Aachen Germany

    Present Address: Department of Mechanical Engineering Imperial College London Exhibition Rd, South Kensington London SW7 2AZ UK

  2. Technical University of Munich

    Affiliation as printed

    School of Engineering & Design Institute of Automotive Technology Technical University of Munich Germany

  3. Jülich Aachen Research Alliance · RWTH Aachen University

    Affiliation as printed

    Chair for Electrochemical Energy Conversion and Storage Systems Institute for Power Electronics and Electrical Drives (ISEA) RWTH Aachen University CampusBoulevard 89 52074 Aachen Germany

    Jülich Aachen Research Alliance JARA-Energy Templergraben 55 52056 Aachen Germany

  4. Jülich Aachen Research Alliance · RWTH Aachen University

    Affiliation as printed

    Chair for Electrochemical Energy Conversion and Storage Systems Institute for Power Electronics and Electrical Drives (ISEA) RWTH Aachen University CampusBoulevard 89 52074 Aachen Germany

    Jülich Aachen Research Alliance JARA-Energy Templergraben 55 52056 Aachen Germany

  5. Jülich Aachen Research Alliance · RWTH Aachen University

    Affiliation as printed

    Chair for Electrochemical Energy Conversion and Storage Systems Institute for Power Electronics and Electrical Drives (ISEA) RWTH Aachen University CampusBoulevard 89 52074 Aachen Germany

    Jülich Aachen Research Alliance JARA-Energy Templergraben 55 52056 Aachen Germany

  6. Technical University of Munich

    Affiliation as printed

    Chair of Electrical Energy Storage Technology Department of Energy and Process Engineering TUM School of Engineering and Design Technical University of Munich Germany

  7. University of Oxford · Jülich Aachen Research Alliance · RWTH Aachen University

    Affiliation as printed

    Chair for Electrochemical Energy Conversion and Storage Systems Institute for Power Electronics and Electrical Drives (ISEA) RWTH Aachen University CampusBoulevard 89 52074 Aachen Germany

    Jülich Aachen Research Alliance JARA-Energy Templergraben 55 52056 Aachen Germany

    Present Address: Department of Engineering Science University of Oxford Parks Road Oxford OX1 3PJ UK

  8. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Thermal Process Engineering (TVT) Karlsruhe Institute of Technology (KIT) Germany

  9. University of Bayreuth

    Affiliation as printed

    Chair of Electrical Energy Systems University of Bayreuth Germany

  10. Technische Hochschule Ingolstadt

    Affiliation as printed

    Research Group Electromobility and Learning Systems THI Ingolstadt Germany

  11. RWTH Aachen University

    Affiliation as printed

    Institute of Statistics RWTH Aachen University Germany

  12. RWTH Aachen University

    Affiliation as printed

    Institute of Statistics RWTH Aachen University Germany

  13. RWTH Aachen University

    Affiliation as printed

    Institute of Statistics RWTH Aachen University Germany

  14. Forschungszentrum Jülich · Jülich Aachen Research Alliance · RWTH Aachen University

    Affiliation as printed

    Chair for Electrochemical Energy Conversion and Storage Systems Institute for Power Electronics and Electrical Drives (ISEA) RWTH Aachen University CampusBoulevard 89 52074 Aachen Germany

    Helmholtz Institute Muenster (HI MS) IEK-12 Forschungszentrum Juelich 52425 Jülich Germany

    Institute for Power Generation and Storage Systems (PGS) E.ON ERC RWTH Aachen University Mathieustrasse 10 52074 Aachen Germany

    Jülich Aachen Research Alliance JARA-Energy Templergraben 55 52056 Aachen Germany

  15. University of Bayreuth

    Affiliation as printed

    Chair of Electrical Energy Systems University of Bayreuth Germany

  16. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Thermal Process Engineering (TVT) Karlsruhe Institute of Technology (KIT) Germany

  17. Technische Hochschule Ingolstadt

    Affiliation as printed

    Research Group Electromobility and Learning Systems THI Ingolstadt Germany

  18. Technical University of Munich

    Affiliation as printed

    School of Engineering & Design Institute of Automotive Technology Technical University of Munich Germany

  19. Technical University of Munich

    Affiliation as printed

    Chair of Electrical Energy Storage Technology Department of Energy and Process Engineering TUM School of Engineering and Design Technical University of Munich Germany

  20. Technische Hochschule Ingolstadt

    Affiliation as printed

    Research Group Electromobility and Learning Systems THI Ingolstadt Germany

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References 265