A climate-optimal supply chain for CO2 capture, utilization, and storage by mineralization

Journal of Cleaner Production, vol. 360, pp. 131750

Abstract

CO2 mineralization not only captures and stores CO2 permanently but also yields value-added products utilized in, for example, the cement industry. CO2 mineralization has been shown to potentially substantially reduce greenhouse gas (GHG) emissions. Realizing CO2 mineralization's potential on a large scale requires a) solid feedstock, b) CO2 sources, c) low-carbon energy, and d) markets for mineralization products. In general, these four requirements of CO2 mineralization are not satisfied at the same location. Thus, the assessment of CO2 mineralization's large-scale potential necessitates the full supply chain considering all requirements for CO2 mineralization simultaneously. At present, neither the potential of CO2 mineralization for GHG emissions reduction on a large scale nor the required supply chain to achieve the potential are fully understood. In our study, we design a climate-optimal supply chain for CO2 capture, utilization, and storage (CCUS) by CO2 mineralization to quantify the large-scale potential of CO2 mineralization in Europe. Our results show that a climate-optimal CCUS by CO2 mineralization could avoid up to 130 Mt CO2e/year of the industrial emissions in Europe even with the current energy supply system. By 2040, CCUS by CO2 mineralization could provide negative emissions of up to 136 Mt CO2e/year. The required energy and CO2 for the CCUS supply chain can be provided either by expanding the current infrastructure by about 5 % or, even more climate efficiently, by building new infrastructure. The critical steps toward achieving the large potential of CO2 mineralization in Europe are 1) scaling up the CO2 mineralization technology to the industrial level and 2) exploiting large-scale mineral deposits.

Authors 4

1. Hesam Ostovari Aachen Institute of Technical Thermodynamics

   RWTH Aachen University

   Affiliation as printed

   Institute of Technical Thermodynamics, RWTH Aachen University, Germany

2. Leonard Jan Müller Aachen Institute of Technical Thermodynamics

   RWTH Aachen University

   Affiliation as printed

   Institute of Technical Thermodynamics, RWTH Aachen University, Germany

3. Fabian Mayer Aachen Institute of Technical Thermodynamics

   RWTH Aachen University · ETH Zurich

   Affiliation as printed

   Energy & Process Systems Engineering, ETH, Zurich, Switzerland

   Institute of Technical Thermodynamics, RWTH Aachen University, Germany

4. André Bardow corresponding Aachen Institute of Technical Thermodynamics

   RWTH Aachen University · ETH Zurich · Forschungszentrum Jülich

   Affiliation as printed

   Energy & Process Systems Engineering, ETH, Zurich, Switzerland

   Institute of Energy and Climate Research - Energy Systems Engineering (IEK-10), Forschungszentrum Jülich GmbH, Jülich, Germany

   Institute of Technical Thermodynamics, RWTH Aachen University, Germany