A

Comment on amt-2021-31

Abstract

Abstract. The thermal infrared nadir spectra of IASI (Infrared Atmospheric Sounding Interferometer) are successfully used for retrievals of different atmospheric trace gas profiles. However, these retrievals offer generally reduced information about the lowermost tropospheric layer due to the lack of thermal contrast close to the surface. Spectra of scattered solar radiation observed in the near-infrared and/or shortwave infrared, for instance by TROPOMI (TROPOspheric Monitoring Instrument), offer higher sensitivity near the ground and are used for the retrieval of total-column-averaged mixing ratios of a variety of atmospheric trace gases. Here we present a method for the synergetic use of IASI profile and TROPOMI total-column level 2 retrieval products. Our method uses the output of the individual retrievals and consists of linear algebra a posteriori calculations (i.e. calculation after the individual retrievals). We show that this approach has strong theoretical similarities to applying the spectra of the different sensors together in a single retrieval procedure but with the substantial advantage of being applicable to data generated with different individual retrieval processors, of being very time efficient, and of directly benefiting from the high quality and most recent improvements of the individual retrieval processors. We demonstrate the method exemplarily for atmospheric methane (CH4). We perform a theoretical evaluation and show that the a posteriori combination method yields a total-column-averaged CH4 product (XCH4) that conserves the good sensitivity of the corresponding TROPOMI product while merging it with the high-quality upper troposphere–lower stratosphere (UTLS) CH4 partial-column information of the corresponding IASI product. As a consequence, the combined product offers additional sensitivity for the tropospheric CH4 partial column, which is not provided by the individual TROPOMI nor the individual IASI product. The theoretically predicted synergetic effect is verified by comparisons to CH4 reference data obtained from collocated XCH4 measurements at 14 globally distributed TCCON (Total Carbon Column Observing Network) stations, CH4 profile measurements made by 36 individual AirCore soundings, and tropospheric CH4 data derived from continuous ground-based in situ observations made at two nearby Global Atmospheric Watch (GAW) mountain stations. The comparisons clearly demonstrate that the combined product can reliably detect the actual variations of atmospheric XCH4, CH4 in the UTLS, and CH4 in the troposphere. A similar good reliability for the latter is not achievable by the individual TROPOMI and IASI products.

Authors 34

  1. Matthias F. Schneider corresponding

    Karlsruhe Institute of Technology · University of Bern · Oeschger Centre for Climate Change Research · Commissariat à l'Énergie Atomique et aux Énergies Alternatives · Laboratoire des Sciences du Climat et de l'Environnement · CEA Paris-Saclay

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

    Laboratoire des Sciences du Climat et de l'Environnement (LSCE), CEA, 91191 Gif-sur-Yvette, France

    now at: Laboratory for the Analysis of Radiocarbon with AMS (LARA), Department of Chemistry, Biochemistry and Pharmaceutical Sciences (DCBP) & Oeschger Centre for Climate Change Research (OCCR), University of Bern, Bern, Switzerland

  2. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

    Steinbuch Centre for Computing (SCC), Karlsruhe Institute of Technology, Karlsruhe, Germany

  3. Karlsruhe Institute of Technology · Tongji University

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

    now at: School of Mechanical Engineering, Tongji University, Shanghai, China

  4. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

    now at: Software Solutions Department, Telespazio Germany GmbH, Darmstadt, Germany

  5. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

  6. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

  7. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

  8. Karlsruhe Institute of Technology

    Affiliation as printed

    Institute of Meteorology and Climate Research (IMK-ASF), Karlsruhe Institute of Technology, Karlsruhe, Germany

  9. Agencia Estatal de Meteorología

    Affiliation as printed

    Izaña Atmospheric Research Center, Agencia Estatal de Meteorología (AEMET), Santa Cruz de Tenerife, Spain

  10. Agencia Estatal de Meteorología

    Affiliation as printed

    Izaña Atmospheric Research Center, Agencia Estatal de Meteorología (AEMET), Santa Cruz de Tenerife, Spain

  11. Space Research Organisation Netherlands

    Affiliation as printed

    Earth Science Group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands

  12. Space Research Organisation Netherlands

    Affiliation as printed

    Earth Science Group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands

  13. Space Research Organisation Netherlands

    Affiliation as printed

    Earth Science Group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands

  14. Heidelberg University

    Affiliation as printed

    Institute of Environmental Physics, Heidelberg University, Heidelberg, Germany

  15. University of Groningen

    Affiliation as printed

    Center for Isotope Research, University of Groningen, Groningen, the Netherlands

  16. Finnish Meteorological Institute

    Affiliation as printed

    Space and Earth Observation Centre, Finnish Meteorological Institute, Sodankylä, Finland

  17. University of Bern · Oeschger Centre for Climate Change Research · Commissariat à l'Énergie Atomique et aux Énergies Alternatives · Laboratoire des Sciences du Climat et de l'Environnement · CEA Paris-Saclay

    Affiliation as printed

    Laboratoire des Sciences du Climat et de l'Environnement (LSCE), CEA, 91191 Gif-sur-Yvette, France

    now at: Laboratory for the Analysis of Radiocarbon with AMS (LARA), Department of Chemistry, Biochemistry and Pharmaceutical Sciences (DCBP) & Oeschger Centre for Climate Change Research (OCCR), University of Bern, Bern, Switzerland

  18. Commissariat à l'Énergie Atomique et aux Énergies Alternatives · Laboratoire des Sciences du Climat et de l'Environnement · CEA Paris-Saclay

    Affiliation as printed

    Laboratoire des Sciences du Climat et de l'Environnement (LSCE), CEA, 91191 Gif-sur-Yvette, France

  19. Centre National de la Recherche Scientifique · École Polytechnique

    Affiliation as printed

    LMD/IPSL, CNRS, École polytechnique, University Paris-Saclay, Palaiseau, France

  20. Centre National de la Recherche Scientifique · École Polytechnique

    Affiliation as printed

    LMD/IPSL, CNRS, École polytechnique, University Paris-Saclay, Palaiseau, France

  21. Swiss Federal Laboratories for Materials Science and Technology

    Affiliation as printed

    Empa, Swiss Federal Laboratories for Materials Science and Technology, Dübendorf, Switzerland

  22. German Environment Agency

    Affiliation as printed

    Air Monitoring Network, Federal Environment Agency (UBA), Langen, Germany

  23. University of Toronto

    Affiliation as printed

    Department of Physics, Universtity of Toronto, Toronto, Canada

  24. University of Toronto

    Affiliation as printed

    Department of Physics, Universtity of Toronto, Toronto, Canada

  25. University of Bremen

    Affiliation as printed

    Institute of Environmental Physics, University of Bremen, Bremen, Germany

  26. California Institute of Technology

    Affiliation as printed

    Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA, USA

  27. California Institute of Technology

    Affiliation as printed

    Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA, USA

  28. National Institute for Environmental Studies

    Affiliation as printed

    Satellite Observation Center, National Institute for Environmental Studies (NIES), Tsukuba, Ibaraki, Japan

  29. Ames Research Center

    Affiliation as printed

    Atmospheric Science Branch, NASA Ames Research Center, Moffett Field, CA, USA

  30. Japan Aerospace Exploration Agency

    Affiliation as printed

    Earth Observation Research Center (EORC), Japan Aerospace Exploration Agency (JAXA), Tsukuba, Japan

  31. University of Wollongong

    Affiliation as printed

    Centre for Atmospheric Chemistry, School of Earth, Atmospheric and Life Sciences, Faculty of Science, Medicine and Health, University of Wollongong, Wollongong, Australia

  32. University of Wollongong

    Affiliation as printed

    Centre for Atmospheric Chemistry, School of Earth, Atmospheric and Life Sciences, Faculty of Science, Medicine and Health, University of Wollongong, Wollongong, Australia

  33. Deutscher Wetterdienst · University of Wollongong

    Affiliation as printed

    Centre for Atmospheric Chemistry, School of Earth, Atmospheric and Life Sciences, Faculty of Science, Medicine and Health, University of Wollongong, Wollongong, Australia

    now at: Meteorological Observatory Hohenpeissenberg, Deutscher Wetterdienst (DWD), Albin-Schwaiger-Weg 10, 82383 Hohenpeissenberg, Germany

  34. National Institute of Water and Atmospheric Research

    Affiliation as printed

    National Institute of Water and Atmospheric Research Ltd (NIWA), Lauder, New Zealand

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References 45