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Charge Transport: Photomodulation of Charge Transport in All‐Semiconducting 2D–1D van der Waals Heterostructures with Suppressed Persistent Photoconductivity Effect (Adv. Mater. 26/2020)

Advanced Materials, vol. 32

Abstract

In article number 2001268, Paolo Samorì and co-workers report the fabrication of all-semiconducting mixed-dimensional van der Waals heterostructures based on monolayer 2D MoS2 and bottom-up synthesized 1D graphene nanoribbons, which efficiently suppress the typical persistent photoconductivity effect of MoS2. Upon interfacing with physisorbed photochromic molecules, the charge transport of MoS2–graphene nanoribbons in field-effect transistors can be significantly photomodulated, which corresponds to multilevel output currents for high-performance optoelectronics.

Authors 11

  1. Centre National de la Recherche Scientifique · Université de Strasbourg · Institut de Science et d'Ingénierie Supramoléculaires

    Affiliation as printed

    University of Strasbourg CNRS ISIS UMR 7006, 8 Alleé Gaspard Monge Strasbourg F‐67000 France

  2. Centre National de la Recherche Scientifique · Université de Strasbourg · Institut de Science et d'Ingénierie Supramoléculaires

    Affiliation as printed

    University of Strasbourg CNRS ISIS UMR 7006, 8 Alleé Gaspard Monge Strasbourg F‐67000 France

  3. Centre National de la Recherche Scientifique · Université de Strasbourg · Institut de Science et d'Ingénierie Supramoléculaires

    Affiliation as printed

    University of Strasbourg CNRS ISIS UMR 7006, 8 Alleé Gaspard Monge Strasbourg F‐67000 France

  4. Max Planck Institute for Polymer Research

    Affiliation as printed

    Max Planck Institute for Polymer Research Ackermannweg 10 Mainz 55128 Germany

    Max Planck Institute for Polymer Research, Ackermannweg 10, Mainz, 55128 Germany

  5. Humboldt-Universität zu Berlin

    Affiliation as printed

    Department of Chemistry and IRIS Adlershof Humboldt‐Universität zu Berlin Berlin 12489 Germany

  6. Max Planck Institute for Polymer Research · Okinawa Institute of Science and Technology Graduate University

    Affiliation as printed

    Max Planck Institute for Polymer Research Ackermannweg 10 Mainz 55128 Germany

    Organic and Carbon Nanomaterials Unit Okinawa Institute of Science and Technology Graduate University 1919‐1 Tancha, Onna‐son, Kunigami Okinawa 904‐0495 Japan

    Max Planck Institute for Polymer Research, Ackermannweg 10, Mainz, 55128 Germany

    Organic and Carbon Nanomaterials Unit, Okinawa Institute of Science and Technology Graduate University, 1919-1 Tancha, Onna-son, Kunigami, Okinawa, 904-0495 Japan

  7. Centre National de la Recherche Scientifique · Université de Strasbourg · Institut de Science et d'Ingénierie Supramoléculaires

    Affiliation as printed

    University of Strasbourg CNRS ISIS UMR 7006, 8 Alleé Gaspard Monge Strasbourg F‐67000 France

  8. RWTH Aachen University · DWI – Leibniz Institute for Interactive Materials · Humboldt-Universität zu Berlin

    Affiliation as printed

    DWI—Leibniz Institute for Interactive Materials Forckenbeckstr. 50 Aachen 52056 Germany

    Department of Chemistry and IRIS Adlershof Humboldt‐Universität zu Berlin Berlin 12489 Germany

    Institute of Technical and Macromolecular Chemistry RWTH Aachen University Worringer Weg 2 Aachen 52074 Germany

    Institute of Technical and Macromolecular Chemistry, RWTH Aachen University, Worringer Weg 2, Aachen, 52074 Germany

  9. Soochow University

    Affiliation as printed

    Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices Institute of Functional Nano & Soft Materials (FUNSOM) Soochow University Suzhou 215123 P. R. China

    Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices Institute of Functional Nano & Soft Materials (FUNSOM) Soochow University Suzhou 215123 P. R. China

  10. Max Planck Institute for Polymer Research

    Affiliation as printed

    Max Planck Institute for Polymer Research Ackermannweg 10 Mainz 55128 Germany

    Max Planck Institute for Polymer Research, Ackermannweg 10, Mainz, 55128 Germany

  11. Centre National de la Recherche Scientifique · Université de Strasbourg · Institut de Science et d'Ingénierie Supramoléculaires

    Affiliation as printed

    University of Strasbourg CNRS ISIS UMR 7006, 8 Alleé Gaspard Monge Strasbourg F‐67000 France

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